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?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>ZIBsQ?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>820 mah/gQ?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>q?/span>?/span>?/span>?/span>(?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>0.76 VQ?/span>?/span>?/span>?/span>Q?/span>ZIBs?/span>?/span>?/span>?/span>?/span>?/span>一?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Zn2 ?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Li {?/span>一?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>q?/span>?/span>?/span>?/span>?/span>?/span>l?/span>?/span>E?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>


q?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>E?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>MOFQ?/span>?/span>p?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>q?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>z?/span>?/span>Q?/span>?/span>?/span>?/span>l?/span>?/span>?/span>?/span>?/span>?/span>一U?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>p?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Coordinately Unsaturated Manganese-Based Metal?/span>Organic Frameworks as a High-Performance Cathode for Aqueous Zinc-Ion Batteries?/span>?/span>?/span>?/span>ACS Applied Materials & Interfaces?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>E?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>W?/span>一?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>-COO-?/span>?/span>?/span>?/span>q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Zn2 ?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>q?/span>E?/span>?/span>?/span>?/span>?/span>?/span>z?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span>?/span>q?/span>?/span>?/span>Q?/span>q?/span>U?/span>?/span>?/span>MOF?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>(?/span>100 mA g-1?/span>?/span>138 mAh g-1)?/span>?/span>?/span>?/span>(?/span>3000 mA g-1?/span>?/span>?/span>1000?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>93.5%)?/span>q?/span>U?/span>?/span>?/span>?/span>Zn2 ?/span>?/span>?/span>?/span>?/span>?/span>?/span>q?/span>?/span>?/span>?/span>?/span>最q?/span>?/span>?/span>?/span>MOF?/span>?/span>?/span>q?/span>U?/span>?/span>q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>p?/span>ZIBs?/span>?/span>?/span>?/span>MOF?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>I?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>{?/span>?/span>?/span>?/span>?/span>?/span>



?/span>1. (a) Mn-H3BTC-MOF-4?/span>Mn(II)?/span>?/span>?/span>q?/span>E?/span>?/span>?/span>?/span>?/span>?/span>C?/span>?/span>?/span>?/span>SEM?/span>?/span>Q?/span>(b,e) Mn-H3BTC-MOF-2Q?/span>(c,f) Mn-H3BTC-MOF-4?/span> (d,g) Mn-H3BTC-MOF-6?/span>



?/span>2. MOFs_?/span>?/span>?/span>C?/span>O?/span>Mn?/span>?/span>?/span>HRTEM?/span>?/span>?/span>EDS?/span>?/span>?/span>?/span>Q?/span>(a) Mn-H3BTC-MOF-2Q?/span>(b) Mn-H3BTC-MOF-4?/span> (c) Mn- H3BTC-MOF-6?/span>



?/span>3. Mn-H3BTC-MOF-2?/span>Mn-H3BTC-MOF-4?/span>Mn-H3BTC-MOF-6?/span> (a-c) XRD?/span>?/span>?/span> (d-f) TGA-DTG?/span>?/span>



?/span>4. ?/span>?/span>?/span>?/span>?/span>FTIR?/span>?/span>Q?/span>(a) Mn-H3BTC-MOF-2Q?/span>(b) Mn-H3BTC-MOF-4Q?/span>(c) Mn-H3BTC-MOF-6?/span> (d) H3BTCQ?/span>?/span>?/span>Mn-H3BTC-MOF-4?/span>?/span>?/span>?/span>?/span> (e) ?/span>?/span>?/span>(f) Mn 2p?/span>(g) O 1s?/span> (h) C 1s XPS?/span>?/span>?/span>



?/span>5. (a) ?/span>?/span>2 M Zn(CF3SO3)2?/span>p?/span>?/span>?/span>?/span>?/span>MOF?/span>?/span>?/span>Zn?/span>?/span>ZIBs?/span>C?/span>?/span>?/span>Q?/span>(b,c) ?/span>?/span>?/span>?/span>?/span> 0.1 mV s?1?/span>?/span>CV?/span>U?/span>?/span>?/span>100 mA g?1?/span>?/span>?/span>?/span>?/span> Q?/span>(d) Mn-H3BTC-MOF-4?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>U?/span>Q?/span>(e) Mn-H3BTC-MOF-4(?/span>100?/span>3000 mA g?1)?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span> (f,g) Mn-H3BTC-MOF-4?/span>?/span>?/span>100?/span>3000 mA g?1?/span>?/span>?/span>?/span>?/span>?/span>?/span>



?/span>6. (a,b) ?/span>?/span>Mn-H3BTC-MOF-4?/span>?/span>?/span>100?/span>?/span>?/span>?/span>?/span>SEM?/span>?/span>?/span>Zn?/span>?/span>?/span>?/span>Q?/span>(c) XRD?/span>?/span>?/span> (d) Mn 2p Q?/span>(e) C 1s?/span> (f) O 1s XPS?/span>?/span>?/span>



?/span>7. ?/span>?/span>?/span>?/span>?/span>?/span>D?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>XRD?/span>?/span>?/span>


?/span>8. (a) Mn-H3BTC-MOF-4?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>CV?/span>U?/span>Q?/span>(b) CV?/span>U?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>log(?/span>?/span>?/span>?/span>)?/span>log(?/span>?/span>?/span>?/span>)?/span>?/span>p?/span>?/span>Q?/span>(c) 0.1 mV s?1?/span>?/span>?/span>?/span>?/span>?/span>(?/span>?/span>?/span>?/span>)?/span>?/span>?/span>?/span>?/span>(?/span>?/span>?/span>?/span>)Q?/span>?/span>?/span> (d) ?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>


?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>一U?/span>?/span>?/span>?/span>?/span>?/span>{?/span>?/span>?/span>?/span>?/span>ZIBs?/span>Mn-H3BTC-MOF-4?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Mn-H3BTC-MOF-2?/span>Mn-H3BTC-MOF-6?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Zn2 ?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>I?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>z?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>I?/span>?/span>?/span>Q?/span>Mn-H3BTC-MOF-4?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>(i) MOFs?/span>?/span>Mn2 ?/span>Zn2 |?/span>?/span>?/span> (ii) Mn2 ?/span>?/span>?/span> MnO2q?/span>?/span>?/span>ZnMn3O7·3H2O?/span>?/span>?/span>?/span>q?/span>U?/span>?/span>?/span>MOF?/span>?/span>?/span>?/span>100 mA g?1?/span>?/span>?/span>138 mAh g?1?/span>?/span>?/span>?/span>?/span>Q?/span>q?/span>?/span>?/span>3000 mA g?1?/span>?/span>?/span>1500?/span>?/span>?/span>?/span>93.5%?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>Q?/span>Mn-H3BTC-MOF-4?/span>Zn2 ?/span>?/span>?/span>?/span>?/span>?/span>?/span>q?/span>?/span>最q?/span>?/span>?/span>?/span>?/span>?/span>?/span>MOF?/span>?/span>?/span>q?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>MOF?/span>?/span>?/span>?/span>?/span>?/span>?/span>?/span>ZIBs?/span>?/span>?/span>?/span>?/span>?/span>?/span>


?/strong>?/strong>?/strong>?/strong>

Chengjie Yin*, Chengling Pan*, Xiaobo Liao, Yusong Pan*, and Liang Yuan*. Coordinately Unsaturated Manganese-Based Metal?/span>Organic Frameworks as a High-Performance Cathode for Aqueous Zinc-Ion Batteries. ACS Appl. Mater. Interfaces

https://doi.org/10.1021/acsami.1c10063

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